Title :
NPC2 , the
protein deficient in Niemann-Pick C2 disease, consists of multiple glycoforms that bind a variety of sterols
Abstract :
- Niemann-Pick C disease is a fatal neurodegenerative disorder characterized by an endolysosomal accumulation of cholesterol and other lipids
- One form of the disease is caused by a deficiency in NPC2 , a soluble lysosomal glycoprotein that binds cholesterol
- To better understand the biological function of NPC2 and how its deficiency results in disease, we have characterized the structural and functional properties of recombinant human protein
- Highly purified NPC2 consists of a complex mixture of glycosylated isoforms , similar to that observed in human brain autopsy specimens
- Mass spectrometric analysis revealed that of the three potential N-linked glycosylation sites present in the mature protein , Asn-19 is not utilized; Asn-39 is linked to an endoglycosidase H (Endo H)-sensitive oligosaccharide, and Asn-116 is variably utilized, either being unmodified or linked to Endo H-sensitive or Endo H-resistant oligosaccharides
- All glycoforms are endocytosed and ameliorate the cholesterol storage phenotype of NPC2-deficient fibroblasts
- In addition, the purified preparation contains a mixture of both free and lipid-bound protein
- All glycoforms bind cholesterol, and sterol binding to NPC2 significantly alters its behavior upon cation-exchange chromatography
- Based on this observation, we developed chromatography-based binding assays and determined that NPC2 forms an equimolar complex with the fluorescent cholesterol analog dehydroergosterol
- In addition, we find that NPC2 binds a range of cholesterol-related molecules (cholesterol precursors , plant sterols, some oxysterols, cholesterol sulfate, cholesterol acetate, and 5-alpha-cholestan-3-one) and that 27-hydroxysterol accumulates in NPC2-deficient mouse liver
- Binding was not detected for various glycolipids, phospholipids, or fatty acids
- These biochemical properties support a direct and specialized function of NPC2 in lysosomal sterol transport
Output (sent_index, trigger,
protein,
sugar,
site):
- 2. glycoprotein, , NPC2, -, -
- 2. glycoprotein, , glycoprotein, -, -
- 4. glycosylated, , isoforms, -, -
- 5. glycosylation, , -, -, sites
- 5. utilized, , -, -, Asn-116
- 5. utilized, , -, -, Asn-19
Output(Part-Of) (sent_index,
protein,
site):
*Output_Site_Fusion* (sent_index,
protein,
sugar,
site):
- 5. NPC2, -, Asn-116
- 5. NPC2, -, Asn-19